Observation of Intervalley Biexcitonic Optical Stark Effect in Monolayer WS2
نویسندگان
چکیده
منابع مشابه
Observation of Intervalley Biexcitonic Optical Stark Effect in Monolayer WS2.
Coherent optical driving can effectively modify the properties of electronic valleys in transition metal dichalcogenides. Here, we observe a new type of optical Stark effect in monolayer WS2, one that is mediated by intervalley biexcitons under the blue-detuned driving with circularly polarized light. We find that such helical optical driving not only induces an exciton energy downshift at the ...
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Breaking space-time symmetries in two-dimensional crystals can markedly influence their macroscopic electronic properties. Monolayer transition metal dichalcogenides (TMDs) are prime examples where the intrinsically broken crystal inversion symmetry permits the generation of valley-selective electron populations, even though the two valleys are energetically degenerate, locked by time-reversal ...
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Semiconductors that are atomically thin can exhibit novel optical properties beyond those encountered in the bulk compounds. Monolayer transition-metal dichalcogenides (TMDs) are leading examples of such semiconductors that possess remarkable optical properties. They obey unique selection rules where light with different circular polarization can be used for selective photoexcitation at two dif...
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ژورنال
عنوان ژورنال: Nano Letters
سال: 2016
ISSN: 1530-6984,1530-6992
DOI: 10.1021/acs.nanolett.6b02998